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結ぶ means "to tie," right? Well, you can see with your eye that something has been tied when it has a knot. The bigger the knot, the easier it is for your eye to see.
This is a combination of the words 結ぶ and 目. If you know how to read those, then you should have no problem with this one.
結び目を作る
to make a knot
結び目をほどく
to untie a knot
結び目をゆるめる
to loosen a knot
結び目を引っぱる
to pull a knot
その固い結び目をほどくのはとても大変だった。
It was very hard to untie the tight knot.
少しだけ結び目をゆるめさせてくださいね。
Please let me loosen the knot a little.
結び目が小さくて見えにくいんだよね。
The knot is small, so it's hard to see, you know?
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